NickelMaghrebV1, France, Analysis, bibRecord, 000207

Ni catalysts from NiAl2O4 spinel for CO2 reforming of methane

Identifieur interne : 000207 ( France/Analysis ); précédent : 000206; suivant : 000208

Ni catalysts from NiAl2O4 spinel for CO2 reforming of methane

Auteurs : N. Sahli [France, Algérie] ; C. Petit [France] ; A. C. Roger [France] ; A. Kiennemann [France] ; S. Libs [France] ; M. M. Bettahar [France]

Source :

Catalysis today [ 0920-5861 ] ; 2006.

RBID : Pascal:06-0371425

Descripteurs français

Pascal (Inist)
- Catalyseur, Spinelle, Spinelles, Reformage, Méthane, Nickel, Gaz synthèse, Catalyse hétérogène, Carbone dioxyde.
Wicri :
- topic : Nickel.

English descriptors

KwdEn :
- Carbon dioxide, Catalyst, Heterogeneous catalysis, Methane, Nickel, Reforming, Spinel, Spinels, Synthesis gas.

Abstract

A series of mixed oxides close to NiAl₂O₄ was obtained by a sol-gel like method (propionic acid). The characterization of the different structures was made by X-ray diffraction (XRD), scanning electron microscopy (SEM) or transmission electron microscopy (TEM). For the stoichiometric ratio of Ni to Al exactly equal to 0.5, homogeneous crystalline spinel phase was formed for a temperature of calcination equal or higher than 725 °C. A solid solution was obtained for a Ni/Al ratio lower than 0.5. The spinel structure is non-tolerant concerning a change of nickel to aluminum ratio higher than 0.5: an excess of nickel gives large particles of NiO on spinel phase. Comparative reduction and dry reforming of these oxides was made to control the formation of Ni and its sintering for applications in methane dry reforming. Preliminary reactivity results in dry reforming of methane are given.

Affiliations:

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to stream Main, to step Merge: 000732
to stream Main, to step Curation: 000713
to stream Main, to step Exploration: 000713
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Pascal:06-0371425

Le document en format XML

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O<sub>4</sub>
 spinel for CO<sub>2</sub>
 reforming of methane</title>
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<sourceDesc><biblStruct><analytic><title xml:lang="en" level="a">Ni catalysts from NiAl<sub>2</sub>
O<sub>4</sub>
 spinel for CO<sub>2</sub>
 reforming of methane</title>
<author><name sortKey="Sahli, N" sort="Sahli, N" uniqKey="Sahli N" first="N." last="Sahli">N. Sahli</name>
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<s2>67087 Strasbourg</s2>
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<s2>67087 Strasbourg</s2>
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<author><name sortKey="Roger, A C" sort="Roger, A C" uniqKey="Roger A" first="A. C." last="Roger">A. C. Roger</name>
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<s2>67087 Strasbourg</s2>
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<author><name sortKey="Kiennemann, A" sort="Kiennemann, A" uniqKey="Kiennemann A" first="A." last="Kiennemann">A. Kiennemann</name>
<affiliation wicri:level="3"><inist:fA14 i1="01"><s1>Ecole Européenne de Chimie, Polymères et Matériaux de Strasbourg-Laboratoire Matériaux, Surface, Procédés Pour la Catalyse UMR 7515-25 Rue Becquerel</s1>
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<author><name sortKey="Libs, S" sort="Libs, S" uniqKey="Libs S" first="S." last="Libs">S. Libs</name>
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<author><name sortKey="Bettahar, M M" sort="Bettahar, M M" uniqKey="Bettahar M" first="M. M." last="Bettahar">M. M. Bettahar</name>
<affiliation wicri:level="3"><inist:fA14 i1="03"><s1>Equipe de Recherche Réactivité et Synthèse Organique, Groupe Catalyse Hétérogène-UMR 7565-Université H. Poincaré, Nancy-1 BP 239</s1>
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<series><title level="j" type="main">Catalysis today</title>
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</fileDesc>
<profileDesc><textClass><keywords scheme="KwdEn" xml:lang="en"><term>Carbon dioxide</term>
<term>Catalyst</term>
<term>Heterogeneous catalysis</term>
<term>Methane</term>
<term>Nickel</term>
<term>Reforming</term>
<term>Spinel</term>
<term>Spinels</term>
<term>Synthesis gas</term>
</keywords>
<keywords scheme="Pascal" xml:lang="fr"><term>Catalyseur</term>
<term>Spinelle</term>
<term>Spinelles</term>
<term>Reformage</term>
<term>Méthane</term>
<term>Nickel</term>
<term>Gaz synthèse</term>
<term>Catalyse hétérogène</term>
<term>Carbone dioxyde</term>
</keywords>
<keywords scheme="Wicri" type="topic" xml:lang="fr"><term>Nickel</term>
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</teiHeader>
<front><div type="abstract" xml:lang="en">A series of mixed oxides close to NiAl<sub>2</sub>
O<sub>4</sub>
 was obtained by a sol-gel like method (propionic acid). The characterization of the different structures was made by X-ray diffraction (XRD), scanning electron microscopy (SEM) or transmission electron microscopy (TEM). For the stoichiometric ratio of Ni to Al exactly equal to 0.5, homogeneous crystalline spinel phase was formed for a temperature of calcination equal or higher than 725 °C. A solid solution was obtained for a Ni/Al ratio lower than 0.5. The spinel structure is non-tolerant concerning a change of nickel to aluminum ratio higher than 0.5: an excess of nickel gives large particles of NiO on spinel phase. Comparative reduction and dry reforming of these oxides was made to control the formation of Ni and its sintering for applications in methane dry reforming. Preliminary reactivity results in dry reforming of methane are given.</div>
</front>
</TEI>
<affiliations><list><country><li>Algérie</li>
<li>France</li>
</country>
<region><li>Alsace (région administrative)</li>
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<name sortKey="Kiennemann, A" sort="Kiennemann, A" uniqKey="Kiennemann A" first="A." last="Kiennemann">A. Kiennemann</name>
<name sortKey="Libs, S" sort="Libs, S" uniqKey="Libs S" first="S." last="Libs">S. Libs</name>
<name sortKey="Petit, C" sort="Petit, C" uniqKey="Petit C" first="C." last="Petit">C. Petit</name>
<name sortKey="Roger, A C" sort="Roger, A C" uniqKey="Roger A" first="A. C." last="Roger">A. C. Roger</name>
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</record>

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Serveur d'exploration sur le nickel au Maghreb

Ni catalysts from NiAl2O4 spinel for CO2 reforming of methane

Ni catalysts from NiAl2O4 spinel for CO2 reforming of methane

Source :

Descripteurs français

English descriptors

Abstract

Links toward previous steps (curation, corpus...)

Links to Exploration step

Le document en format XML

Pour manipuler ce document sous Unix (Dilib)

Pour mettre un lien sur cette page dans le réseau Wicri